Anti-Stokes Raman Scattering of Single Carbyne Chains
dc.contributor.author
Tschannen, Cla Duri
dc.contributor.author
Frimmer, Martin
dc.contributor.author
Gordeev, Georgy
dc.contributor.author
Vasconcelos, Thiago L.
dc.contributor.author
Shi, Lei
dc.contributor.author
Pichler, Thomas
dc.contributor.author
Reich, Stephanie
dc.contributor.author
Heeg, Sebastian
dc.contributor.author
Novotny, Lukas
dc.date.accessioned
2021-08-04T06:23:52Z
dc.date.available
2021-07-15T12:05:04Z
dc.date.available
2021-07-15T12:48:50Z
dc.date.available
2021-08-04T06:23:52Z
dc.date.issued
2021-07-27
dc.identifier.issn
1936-0851
dc.identifier.issn
1936-086X
dc.identifier.other
10.1021/acsnano.1c03893
en_US
dc.identifier.uri
http://hdl.handle.net/20.500.11850/495359
dc.identifier.doi
10.3929/ethz-b-000495359
dc.description.abstract
We investigate the anti-Stokes Raman scattering of single carbyne chains confined inside double-walled carbon nanotubes. Individual chains are identified using tip-enhanced Raman scattering (TERS) and heated by resonant excitation with varying laser powers. We study the temperature dependence of carbyne’s Raman spectrum and quantify the laser-induced heating based on the anti-Stokes/Stokes ratio. Due to its molecular size and its large Raman cross section, carbyne holds great promise for local temperature monitoring, with potential applications ranging from nanoelectronics to biology.
en_US
dc.format
application/pdf
en_US
dc.language.iso
en
en_US
dc.publisher
American Chemical Society
dc.rights.uri
http://creativecommons.org/licenses/by/4.0/
dc.subject
carbyne
en_US
dc.subject
linear carbon chains
en_US
dc.subject
Raman scattering
en_US
dc.subject
TERS
en_US
dc.subject
Raman thermometry
en_US
dc.subject
anti-Stokes
en_US
dc.subject
nanometrology
en_US
dc.title
Anti-Stokes Raman Scattering of Single Carbyne Chains
en_US
dc.type
Journal Article
dc.rights.license
Creative Commons Attribution 4.0 International
dc.date.published
2021-07-13
ethz.journal.title
ACS Nano
ethz.journal.volume
15
en_US
ethz.journal.issue
7
en_US
ethz.journal.abbreviated
ACS Nano
ethz.pages.start
12249
en_US
ethz.pages.end
12255
en_US
ethz.version.deposit
publishedVersion
en_US
ethz.grant
Antenna-coupled Optoelectronics
en_US
ethz.identifier.wos
ethz.identifier.scopus
ethz.publication.place
Washington, DC
ethz.publication.status
published
en_US
ethz.leitzahl
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02140 - Dep. Inf.technologie und Elektrotechnik / Dep. of Inform.Technol. Electrical Eng.::03944 - Novotny, Lukas / Novotny, Lukas
en_US
ethz.leitzahl.certified
ETH Zürich::00002 - ETH Zürich::00012 - Lehre und Forschung::00007 - Departemente::02140 - Dep. Inf.technologie und Elektrotechnik / Dep. of Inform.Technol. Electrical Eng.::03944 - Novotny, Lukas / Novotny, Lukas
en_US
ethz.grant.agreementno
192362
ethz.grant.fundername
SNF
ethz.grant.funderDoi
10.13039/501100001711
ethz.grant.program
Projekte MINT
ethz.relation.isSupplementedBy
10.3929/ethz-b-000495532
ethz.date.deposited
2021-07-15T12:05:10Z
ethz.source
FORM
ethz.eth
yes
en_US
ethz.availability
Open access
en_US
ethz.rosetta.installDate
2021-08-04T06:24:19Z
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2024-02-02T14:28:13Z
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Publikationstyp
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Journal Article [130173]